What we do...

Our experimental work focuses on light-based sensing technologies which have applications in healthcare diagnostics, environmental monitoring and homeland security. We also use light-based techniques to analyse painted art-works without damaging them. In our computational work, we employ advanced computer-modelling techniques to 'design' and understand the physical behaviour of functional materials, such as new computer-memory materials.

We are funded by...

We are grateful to NIHR (i4i) and EPSRC for funding these projects.

Our research

Our research is mainly concerned with different aspects of (bio)chemical sensing (e.g. using MEMS or optical devices), and with non-crystalline materials (e.g. glasses), understanding their physical properties in terms of their atomic structure and defects. The approach is multidisciplinary, covering solid-state chemistry, physics and materials science. Areas of interest include:

  • Microcantilever sensors for ultra-sensitive detection of chemical and biological analytes.
  • Optical sensors, including evanescent-waveguide sensors, SERS using holographic substrates.
  • Computer simulation of the atomic structure and vibrational dynamics of disordered materials.
  • Ab-initio computer simulation of phase transformations and optically-induced metastabilities in glasses, e.g. used in phase-change memories (Flash replacement).
  • Experimental study of optically-induced changes in glasses, with applications in the fields of optical- waveguides and chemical sensors, data storage and all-optical actuation.

Figure: Ab initio molecular-dynamics model of the amorphous state of the phase-change non- volatile memory material Ge2Sb2Te5

Selected Publications

 

  • Computer-simulation design of new phase-change memory materials. Phys. Status Solidi A 207, 510 (2010)
  • Spatial distribution of rare-earth ions and GaS4 tetrahedra in chalcogenide glasses studied via laser spectroscopy and ab initio molecular dynamics simulation. Phys. Rev. B 81, 104204 (2010)
  • Simultaneous readout of multiple microcantilever arrays with phase-shifting interferometric microscopy (PSIM) Rev. Sci. Instr. (2009), 80, 093101-8
  • Evidence of formation of tightly bound rare-earth clusters in chalcogenide glasses and their evolution with glass compositions. Phys Rev B, (2009), 79, 180202(1-4)
  • Evanescent-Wave Excitation of Surface-Enhanced Raman Scattering Substrates by an Optical-Fiber Taper. Optics Letters (2009) 34, 2685-2687
  • Microscopic origin of the fast crystallization ability of Ge-Sb-Te phase-change memory materials, Nat. Mat., (2008), 7, 399
  • All-optical actuation of amorphous chalcogenide-coated cantilevers, J. Non-Cryst. Sol., (2007), 353, 250.
  • Universal features of terahertz absorption in disordered materials, Phys. Rev. Lett., (2006), 97, 055504
  • Universal features of localized eigenstates in disordered systems, J. Phys. Cond. Matt, (2005), 17, L321

Publications

Preferred orientation of nanoscale order at the surface of amorphous Ge2Sb2Te5 films
T Tony Li, T Hoon Lee, SR Elliott, JR Abelson
Applied Physics Letters
(2013)
103
Near‐field optical enhancement by lead‐sulfide quantum dots and metallic nanoparticles for SERS
T Hutter, S Mahajan, SR Elliott
Journal of Raman Spectroscopy
(2013)
44
Near‐field optical enhancement by lead‐sulfide quantum dots and metallic nanoparticles for SERS
T Hutter, S Mahajan, SR Elliott
Journal of Raman Spectroscopy
(2013)
44
Origin of the unusual reflectance and density contrasts in the phase-change material Cu2GeTe3
JM Skelton, K Kobayashi, Y Sutou, SR Elliott
Applied Physics Letters
(2013)
102
Selective detection of tetrahedral units in amorphous GeTe-based phase change alloys using Ge L3-edge x-ray absorption near-edge structure spectroscopy (vol 102, 111904, 2013)
M Krbal, AV Kolobov, P Fons, KV Mitrofanov, Y Tamenori, J Hegedus, SR Elliott, J Tominaga
Applied Physics Letters
(2013)
102
In silico optimization of phase-change materials for digital memories: a survey of first-row transition-metal dopants for Ge₂Sb₂Te₅.
JM Skelton, SR Elliott
Journal of Physics Condensed Matter
(2013)
25
Near-Field Plasmonics of an Individual Dielectric Nanoparticle above a Metallic Substrate
T Hutter, FM Huang, SR Elliott, S Mahajan
Journal of Physical Chemistry C
(2013)
117
Multivariate analysis of combined Raman and fibre-optic reflectance spectra for the identification of binder materials in simulated medieval paints
A Pallipurath, J Skelton, P Ricciardi, S Bucklow, S Elliott
Journal of Raman Spectroscopy
(2013)
44
Multivariate analysis of combined Raman and fibre-optic reflectance spectra for the identification of binder materials in simulated medieval paints
A Pallipurath, J Skelton, P Ricciardi, S Bucklow, S Elliott
Journal of Raman Spectroscopy
(2013)
44
PCB-integrated optical waveguide sensors: An ammonia gas sensor
N Bamiedakis, T Hutter, RV Penty, IH White, SR Elliott
Journal of Lightwave Technology
(2013)
31

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